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2 days ago · Yifan Zhang. School of Environmental and Chemical Engineering, Shanghai University, 99 Shangda Road, Shanghai, 200444 China. Search for more papers by this author.
3 days ago · Despite extensive studies, how carrier-protein-independent BesD dictates the reaction toward thermodynamically unfavored halogenation is still elusive. Here, we investigated the chlorination versus hydroxylation selectivity in both carrier-protein-independent halogenase BesD and hydroxylase-evolved halogenase Chi-14, employing extensive MD simulations and QM/MM calculations. In BesD, our ...
4 days ago · Haiting Zhang 1, Yifan Qian 1, Zhen-Xia Niu 1,*, and Qian Wang 1,2,† 1 Department of Physics, Zhejiang Normal University, Jinhua 321004, China; 2 CAMTP-Center for Applied Mathematics and Theoretical Physics, University of Maribor, Mladinska 3, SI-2000, Maribor, Slovenia * niuzhx@zjnu.edu.cn † qwang@zjnu.edu.cn
4 days ago · TiO2-based catalysts with various surface heterostructures (0D, 1D, 2D, and 3D) have been widely researched owing to their cost-effectiveness, high stability, and environmentally friendly nature, and can be used for many applications in various fields, including hydrogen production and pollutant degradation. However, there are also many existing problems limiting their practical application ...
1 day ago · Yunfei Wei, Yifan Xu, Hongbo Zhang, Jingyun Jiang and Qun Xu Abstract Anion-regulated two-dimensional amorphous bi-metallic NiFe nitrides are fabricated by annealing controllable NiFe complexes in the rational deep eutectic solvents.
3 days ago · @article{Zhang2024ConformationalIO, title={Conformational Isomerization of the Fe(III)–OH Species Enables Selective Halogenation in Carrier-Protein-Independent Halogenase BesD and Hydroxylase-Evolved Halogenase}, author={Jinyan Zhang and Yifan Li and Wenli Yuan and Xuan Zhang and Yubing Si and Binju Wang}, journal={ACS Catalysis}, year={2024 ...
2 days ago · The hierarchical design liberates the MLLM from low-level control signal decoding and therefore fully releases their emergent capability in high-level perception, reasoning, and planning. We build a new dataset with action hierarchy annotations. Comprehensive closed-loop evaluations demonstrate several key advantages of our proposed AD-H system.
