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- Season 5 overviewSep 26, 1969-May 15, 197026 episodesSeason 5 episodes1. Pheasant Under Glass Sep 26, 1969
- Max and 99 must rescue Professor Milo Pheasant, who is being held captive by KAOS agents.
- 2. Ironhand Oct 3, 1969
- Smart must go to Washington to get secret plans when his contact is killed.
- 3. Valerie of the Dolls Oct 10, 1969
- Max intercepts part of a formula for a deadly explosive KAOS is creating.
- 4. Widow Often Annie Oct 17, 1969
- Max romances a KAOS agent, all in the line of duty, of course.
- 5. The Treasure of C. Errol Madre Oct 24, 1969
- Smart seeks a lost gold mine; KAOS robs CONTROL and has financial problems.
- 6. Smart Fell on Alabama Oct 31, 1969
- Max must switch a code-key document for a fake without KAOS catching on.
- 7. And Baby Makes Four Nov 7, 1969
- Max prepares for the arrival of his first-born amidst the chaos of a plan to thwart KAOS.
- 8. And Baby Makes Four Nov 14, 1969
- Max takes 99 to KAOS headquarters by mistake when she starts labor pains.
- 9. Physician Impossible Nov 21, 1969
- Max is mistaken for a doctor by KAOS agents who need a doctor to remove a bullet.
- 10. The Apes of Wrath Nov 28, 1969
- A banana through the mail spells death for the CONTROL agent who receives it.
- 11. Age Before Duty Dec 5, 1969
- KAOS invents a new instant aging process and 15 CONTROL agents die of old age.
- 12. Is This Trip Necessary? Dec 12, 1969
- A KAOS mad scientist develops a new hallucinogenic drug and demands $50,000.
- 13. Ice Station Siegfried Dec 19, 1969
- Agent 99 and CIA agent Quigley must save the world from a mad scientist who is freezing it.
- 14. Moonlighting Becomes You Jan 2, 1970
- Agent 99 infiltrates a radio program to learn the identity of a KAOS agent.
- 15. House of Max Jan 9, 1970
- While in London, Max and 99 try to find out who is recreating "Jack the Ripper" type murders.
- 16. House of Max Jan 16, 1970
- A scientist has created a serum to bring wax figures to life, and he starts with Jack the Ripper.
- 17. Rebecca of Funny-Folk Farm Jan 23, 1970
- When Smart accidentally jettisons a secret package from a plane, he has to retrieve it.
- 18. The Mess of Adrian Listenger Jan 30, 1970
- Max and the Chief each suspect the other of murdering seven CONTROL agents.
- 19. Witness for the Execution Feb 6, 1970
- Max is assigned to protect a KAOS agent who is defecting to CONTROL.
- 20. How Green Was My Valet Feb 13, 1970
- Max is assigned to retrieve a bottle of a new type of liquid rocket fuel.
- 21. And Only Two Ninety-Nine Feb 20, 1970
- Agent 99 is kidnapped and replaced with an exact duplicate by KAOS; the Chief wants to know why.
- 22. Smartacus Feb 27, 1970
- Max and the Chief try to find out how KAOS is gathering secret information.
- 23. What's It All About, Algie? Apr 24, 1970
- Max gets a job at a nursery where one CONTROL agent has already mysteriously disappeared.
- 24. Hello Columbus, Goodbye America May 1, 1970
- Max is astonished to learn that the United States belongs to the direct descendant of Columbus.
- 25. Do I Hear a Vaults? May 8, 1970
- Agent Maxwell Smart locks the Chief and Larrabee inside of a vault.
- 26. I Am Curiously Yellow May 15, 1970
- Agent Maxwell Smart falls prey to a KAOS plot to hypnotize CONTROL agents.