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- Season 2 overviewSep 17, 1966-Apr 22, 196730 episodesSeason 2 episodes1. Anatomy of a Lover Sep 17, 1966
- Max and 99 search for a KAOS agent who reprogrammed Hymie the robot.
- 2. Strike While the Agent Is Hot Sep 24, 1966
- Max becomes the head of the Guild of Surviving CONTROL Agents.
- 3. A Spy for a Spy Oct 1, 1966
- Max and a KAOS kingpin start a kidnap spree to exchange prisoners.
- 4. The Only Way to Die Oct 8, 1966
- Max is wounded and 99 assumes he's dead when the "Blaster" comes back to town.
- 5. Maxwell Smart, Alias Jimmy Ballantine Oct 15, 1966
- Agent Maxwell Smart poses as a safecracker who is employed by KAOS.
- 6. Casablanca Oct 22, 1966
- Agent 99 is sent to Casablanca to find the murderer of 275 top scientists.
- 7. The Decoy Oct 29, 1966
- KAOS breaks the CONTROL code and Max is sent on a suicide mission as a decoy.
- 8. Hoo Done It Nov 5, 1966
- Max, 99 and Harry Hoo are left on a deserted Pacific island to look for a mysterious murderer.
- 9. Rub-a-Dub-Dub, Three Spies in a Sub Nov 12, 1966
- Max and 99 are assigned a suicide mission to destroy a KAOS computer.
- 10. The Greatest Spy on Earth Nov 19, 1966
- Max and 99 are discovered as CONTROL agents while investigating a circus.
- 11. Island of the Darned Nov 26, 1966
- Max and 99 are the prey as they are pursued by a KAOS agent on a Caribbean island.
- 12. Bronzefinger Dec 3, 1966
- Max and 99 try to trap a KAOS agent who forges famous paintings.
- 13. Perils in a Pet Shop Dec 10, 1966
- Max, 99 and Fang go to a pet store which they suspect is a front for KAOS.
- 14. The Whole Tooth And ... Dec 24, 1966
- Only Max knows who has the secret plans needed to keep a reactor from exploding.
- 15. Kiss of Death Dec 31, 1966
- Max comes to the rescue of a madcap heiress who staged her own kidnapping.
- 16. It Takes One to Know One Jan 7, 1967
- CONTROL pits their robot, Hymie, against KAOS' notorious killer, Octavia.
- 17. Someone Down Here Hates Me Jan 14, 1967
- Max learns he is number one on the KAOS kill list with a bounty on his head.
- 18. Cutback at CONTROL Jan 21, 1967
- Max joins KAOS in an attempt to find out who's paying off CONTROL agents.
- 19. The Mummy Jan 28, 1967
- Max is assigned to solve the mysterious disappearance of CONTROL agents.
- 20. The Girls From KAOS Feb 4, 1967
- KAOS wants to kidnap Miss U.S.A. in an attempt to get her scientist father to cooperate with them.
- 21. The Man From YENTA Feb 11, 1967
- Max and 99 must find the KAOS agent who has infiltrated the harem of an important prince.
- 22. Smart Fit the Battle of Jericho Feb 18, 1967
- Max must learn how KAOS is able to blow up every building used for the space program.
- 23. Where-What-How-Who Am I? Feb 25, 1967
- Max learns of KAOS' plans to kill top space scientists, but crashes his car on the way to CONTROL.
- 24. The Expendable Agent Mar 4, 1967
- KAOS plants a bomb in Max's apartment to kill a visiting scientist.
- The KAOS leader, Siegfried, plans the world's biggest kidnapping scheme.
- 26. Appointment in Sahara Mar 25, 1967
- KAOS blackmails the world by threatening to launch a missile.
- 27. Pussycats Galore Apr 1, 1967
- Max and 99 are caught and readied to be shipped behind the Iron Curtain.
- 28. A Man Called Smart Apr 8, 1967
- An important informant is wounded before he can tell Max about a secret formula.
- 29. A Man Called Smart Apr 15, 1967
- KAOS blackmails the entire nation with the dehydration formula.
- 30. A Man Called Smart Apr 22, 1967
- KAOS starts drying up the United States with a secret formula.