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- Season 4 overviewSep 21, 1968-Apr 12, 196926 episodesSeason 4 episodes1. The Impossible Mission Sep 21, 1968
- Max and 99 must retrieve a deadly scientific theory from KAOS.
- 2. Snoopy Smart Versus the Red Baron Sep 28, 1968
- KAOS threatens to wipe out the potato crop by dusting from the air.
- 3. Closely Watched Planes Oct 5, 1968
- Max and 99 try to learn how couriers have been disappearing into thin air.
- 4. The Secret of Sam Vittorio Oct 12, 1968
- CONTROL substitutes Smart and 99 look-alikes for the cronies of a bank robber.
- 5. Diamonds Are a Spy's Best Friend Oct 19, 1968
- Max unknowingly stumbles onto a KAOS robbery unit specializing in diamonds.
- 6. The Worst Best Man Oct 26, 1968
- It seems that every man Max picks as his best man meets with a mysterious accident.
- 7. The Return of the Ancient Mariner Nov 9, 1968
- Max has all kinds of trouble hunting for KAOS agent "The Chameleon.".
- 8. With Love and Twitches Nov 16, 1968
- Max has to fight his way to the altar to be on time for his wedding.
- 9. The Laser Blazer Nov 30, 1968
- Smart's new maid is more than she seems, and 99 and the Chief help Max to realize it.
- 10. The Farkas Fracas Dec 7, 1968
- Max and the Chief almost fall prey to a KAOS plot to photograph important papers.
- 11. Temporarily Out of CONTROL Dec 14, 1968
- Their efforts to get ashore put both Max and the chief in the brig.
- 12. Schwartz's Island Dec 21, 1968
- The Smarts' honeymoon is delayed by a KAOS plot to sabotage the American fleet.
- 13. One Nation Invisible Dec 28, 1968
- Max and 99 have a misunderstanding over a beautiful scientist.
- 14. Hooray for Hollywood Jan 4, 1969
- Max and 99 are assigned to find a KAOS communications system.
- 15. The Day They Raided the Knights Jan 11, 1969
- Agent 99 is surprised to suddenly discover that she is working for KAOS.
- 16. Tequila Mockingbird Jan 18, 1969
- Agent Maxwell Smart and Agent 99 search for hidden gems in Mexico.
- 17. I Shot 86 Today Feb 1, 1969
- The Smarts learn that KAOS plans to blow up a CONTROL building at a specific time.
- 18. Absorb the Greek Feb 8, 1969
- The Smarts think that the Chief has gone daft when he risks romancing a beautiful woman.
- 19. To Sire, With Love Feb 15, 1969
- Agent Maxwell Smart must pose as his look-alike, King Charles.
- 20. To Sire, With Love Feb 22, 1969
- The chief decides to hide King Charles by posing him as Agent Smart.
- 21. Shock It to Me Mar 1, 1969
- A mad scientist plots to send Max and 99 into a five-year sleep.
- 22. Leadside Mar 8, 1969
- Smart is squared off against the infamous Leadside and his assistants.
- 23. Greer Window Mar 15, 1969
- Max's personal snooping leads to a clue about a KAOS research lab.
- 24. The Not-So-Great Escape Mar 15, 1969
- Agent Maxwell Smart starts an investigation into a series of abductions.
- 25. The Not-So-Great Escape Mar 22, 1969
- The Chief suspects an informer is in the midst of the prisoners.
- 26. A Tale of Two Tails Apr 12, 1969
- Max gives an easy assignment to two pupils -- follow 99 while she's shopping.